Changeset 4358


Ignore:
Timestamp:
Mar 11, 2020 4:35:38 AM (4 years ago)
Author:
vondreele
Message:

update tutorial

Location:
Tutorials/RMCProfile-II
Files:
52 added
52 deleted
2 edited

Legend:

Unmodified
Added
Removed

  • Tutorials/RMCProfile-II/RMCProfile-II.htm

    r4329 r4358  
    2323  <o:Author>vondreele</o:Author>
    2424  <o:LastAuthor>vondreele</o:LastAuthor>
    25   <o:Revision>12</o:Revision>
    26   <o:TotalTime>3686</o:TotalTime>
     25  <o:Revision>13</o:Revision>
     26  <o:TotalTime>3712</o:TotalTime>
    2727  <o:Created>2020-02-25T13:19:00Z</o:Created>
    28   <o:LastSaved>2020-02-26T14:20:00Z</o:LastSaved>
    29   <o:Pages>34</o:Pages>
    30   <o:Words>4324</o:Words>
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     28  <o:LastSaved>2020-03-11T09:35:00Z</o:LastSaved>
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    … …  
    12111211<div class=WordSection1>
    12121212
    1213 <h1><span class=SpellE><span style='mso-fareast-font-family:"Times New Roman"'>RMCProfile</span></span><span
    1214 style='mso-fareast-font-family:"Times New Roman"'> – II<o:p></o:p></span></h1>
     1213<h1><span style='mso-fareast-font-family:"Times New Roman"'>RMCProfile – II<o:p></o:p></span></h1>
    12151214
    12161215<h2><span style='mso-fareast-font-family:"Times New Roman"'>Introduction<o:p></o:p></span></h2>
    12171216
    12181217<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>In
    1219 this tutorial, we will show how to use GSAS-II in conjunction with <span
    1220 class=SpellE>RMCProfile</span> (“<span class=SpellE>RMCProfile</span>: Reverse
    1221 Monte Carlo for polycrystalline materials”, M.G. Tucker, D.A. Keen, M.T. Dove,
    1222 A.L. Goodwin and Q. Hui, (2007) Jour. Phys.: Cond. Matter, <b style='mso-bidi-font-weight:
    1223 normal'>19</b>, 335218. <span class=SpellE>doi</span>: <a
     1218this tutorial, we will show how to use GSAS-II in conjunction with RMCProfile
     1219(“RMCProfile: Reverse Monte Carlo for polycrystalline materials”, M.G. Tucker,
     1220D.A. Keen, M.T. Dove, A.L. Goodwin and Q. Hui, (2007) Jour. Phys.: Cond.
     1221Matter, <b style='mso-bidi-font-weight:normal'>19</b>, 335218. <span
     1222class=SpellE>doi</span>: <a
    12241223href="https://doi.org/10.1088/0953-8984/19/33/335218">https://doi.org/10.1088/0953-8984/19/33/335218</a>)
    12251224to fit both neutron powder diffraction data and a pair distribution function
    … …  
    12291228
    12301229<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>Before
    1231 getting started you must have the most recent Version 6 of the <span
    1232 class=SpellE>RMCProfile</span> executable (at this writing this is <span
    1233 class=SpellE>RMCProfile</span> V6.7.6 Beta Serial). Obtain this from <a
    1234 href="http://www.rmcprofile.org">www.rmcprofile.org</a> by following the
    1235 prompts from Downloads. This version is available for Windows, Mac OSX and
     1230getting started you must have the most recent Version 6 of the RMCProfile
     1231executable (at this writing this is RMCProfile V6.7.6 Beta Serial). Obtain this
     1232from <a href="http://www.rmcprofile.org">www.rmcprofile.org</a> by following
     1233the prompts from Downloads. This version is available for Windows, Mac OSX and
    12361234Linux. The download will be a zip file; save it somewhere convenient. Pull from
    12371235it only the </span><span class=SpellE><span class=SubtitleChar><span
    … …  
    12401238style='mso-fareast-font-family:"Times New Roman"'> and place it in the GSASII
    12411239main directory or in a new subdirectory (e.g. </span><span class=SubtitleChar><span
    1242 style='font-size:11.0pt'>GSASII/<span class=SpellE>RMCProfile</span></span></span><span
    1243 style='mso-fareast-font-family:"Times New Roman"'>); no other files are needed
    1244 although you may wish to also retrieve the contents of the tutorial
    1245 subdirectory. It contains </span><span class=SubtitleChar><span
    1246 style='font-size:11.0pt'>rmcprofilemanual.pdf</span></span><span
     1240style='font-size:11.0pt'>GSASII/RMCProfile</span></span><span style='mso-fareast-font-family:
     1241"Times New Roman"'>); no other files are needed although you may wish to also
     1242retrieve the contents of the tutorial subdirectory. It contains </span><span
     1243class=SubtitleChar><span style='font-size:11.0pt'>rmcprofilemanual.pdf</span></span><span
    12471244style='mso-fareast-font-family:"Times New Roman"'> and </span><span
    12481245class=SubtitleChar><span style='font-size:11.0pt'>rmcprofile_tutorial.pdf</span></span><span
    12491246style='mso-fareast-font-family:"Times New Roman"'> which may be of interest
    1250 since the GSAS-II/<span class=SpellE>RMCProfile</span> tutorials are based on
    1251 the latter.<o:p></o:p></span></p>
     1247since the GSAS-II/RMCProfile tutorials are based on the latter.<o:p></o:p></span></p>
    12521248
    12531249<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'><o:p>&nbsp;</o:p></span></p>
    12541250
    12551251<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>The
    1256 process for using <span class=SpellE>RMCProfile</span> begins with a normal
    1257 Rietveld refinement of the average structure. For the kind of disordered
    1258 materials of interest here, this may give bond lengths that are frequently too
    1259 short for the atoms involved and sometimes extreme apparent thermal motion for
    1260 some of the atoms. These effects arise because the average structure places
    1261 these atoms too close to one another; a more localized view would show
    1262 coordinated atom displacements or reorientation of groups of atoms to avoid the
    1263 close contacts. <span class=SpellE>RMCProfile</span> is then used to
    1264 characterize these local displacements by fitting to the diffraction data and
    1265 its Fourier transform as a PDF.<o:p></o:p></span></p>
     1252process for using RMCProfile begins with a normal Rietveld refinement of the
     1253average structure. For the kind of disordered materials of interest here, this
     1254may give bond lengths that are frequently too short for the atoms involved and
     1255sometimes extreme apparent thermal motion for some of the atoms. These effects
     1256arise because the average structure places these atoms too close to one
     1257another; a more localized view would show coordinated atom displacements or
     1258reorientation of groups of atoms to avoid the close contacts. RMCProfile is
     1259then used to characterize these local displacements by fitting to the
     1260diffraction data and its Fourier transform as a PDF.<o:p></o:p></span></p>
    12661261
    12671262<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'><o:p>&nbsp;</o:p></span></p>
    12681263
    12691264<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>The
    1270 material used in this tutorial is the same as described in the <span
    1271 class=SpellE>RMCProfile</span> tutorial Exercise 4, strontium <span
    1272 class=SpellE>titanate</span> (SrTiO<sub>3</sub>). In this perovskite the TiO6
    1273 octahedra are slightly tilted to accommodate the <span class=SpellE>Ti</span>-O
    1274 bond length in a slightly too small unit cell. The data used here was obtained
    1275 at 190K on the GEM diffractometer at ISIS, Rutherford-Appleton Laboratory, <span
    1276 class=GramE>Harwell</span> Campus, UK. The process of creating this data
    1277 introduced two minor flaws: one is a slight <span class=SpellE>mis</span>-scaling
    1278 of the magnitudes of the real space, G(R), and reciprocal space, F(Q), patterns
    1279 and the other is a difference in the diffractometer constant, <span
    1280 class=SpellE>difC</span>, used to make them vs that used for the Rietveld
    1281 refinement. In this tutorial we will address both of these in case you
    1282 encounter them in your future work with <span class=SpellE>RMCProfile</span>.<o:p></o:p></span></p>
     1265material used in this tutorial is the same as described in the RMCProfile
     1266tutorial Exercise 4, strontium <span class=SpellE>titanate</span> (SrTiO<sub>3</sub>).
     1267In this perovskite the TiO6 octahedra are slightly tilted to accommodate the <span
     1268class=SpellE>Ti</span>-O bond length in a slightly too small unit cell. The
     1269data used here was obtained at 190K on the GEM diffractometer at ISIS,
     1270Rutherford-Appleton Laboratory, <span class=GramE>Harwell</span> Campus, UK.
     1271The process of creating this data introduced two minor flaws: one is a slight <span
     1272class=SpellE>mis</span>-scaling of the magnitudes of the real space, G(R), and
     1273reciprocal space, F(Q), patterns and the other is a difference in the
     1274diffractometer constant, <span class=SpellE>difC</span>, used to make them vs
     1275that used for the Rietveld refinement. In this tutorial we will address both of
     1276these in case you encounter them in your future work with RMCProfile.<o:p></o:p></span></p>
    12831277
    12841278<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'><o:p>&nbsp;</o:p></span></p>
    … …  
    13121306style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
    13131307mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>xye</span></b></span>
    1314 format (angles in degrees) used by <span class=SpellE>topas</span>, etc. to see
    1315 them. Because you used <span style='mso-fareast-font-family:Calibri;mso-fareast-theme-font:
    1316 minor-latin'>the </span><b style='mso-bidi-font-weight:normal'><span
    1317 style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
    1318 mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin;mso-hansi-theme-font:
    1319 minor-latin'>Help/Download tutorial</span></b><span style='mso-fareast-font-family:
    1320 Calibri;mso-fareast-theme-font:minor-latin'> menu entry to open this page and
    1321 downloaded the exercise files (recommended), then the </span><span
    1322 class=SpellE><b style='mso-bidi-font-weight:normal'><span style='font-family:
     1308format to see them. Because you used <span style='mso-fareast-font-family:Calibri;
     1309mso-fareast-theme-font:minor-latin'>the </span><b style='mso-bidi-font-weight:
     1310normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
     1311minor-latin;mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin;
     1312mso-hansi-theme-font:minor-latin'>Help/Download tutorial</span></b><span
     1313style='mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin'>
     1314menu entry to open this page and downloaded the exercise files (recommended),
     1315then the </span><b style='mso-bidi-font-weight:normal'><span style='font-family:
    13231316"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;mso-fareast-font-family:
    1324 Calibri;mso-fareast-theme-font:minor-latin;mso-hansi-theme-font:minor-latin'>RMCProfile</span></b></span><b
    1325 style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
    1326 mso-ascii-theme-font:minor-latin;mso-fareast-font-family:Calibri;mso-fareast-theme-font:
    1327 minor-latin;mso-hansi-theme-font:minor-latin'>-II/data/...</span></b><span
     1317Calibri;mso-fareast-theme-font:minor-latin;mso-hansi-theme-font:minor-latin'>RMCProfile-II/data/...</span></b><span
    13281318style='mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin'>
    13291319entry will bring you to the location where the files have been downloaded. (It
    … …  
    13891379 <v:imagedata src="RMCProfile-II_files/image086.png" o:title=""/>
    13901380</v:shape><![endif]--><![if !vml]><img border=0 width=235 height=320
    1391 src="RMCProfile-II_files/image017.gif" v:shapes="Picture_x0020_45"><![endif]></span><span
     1381src="RMCProfile-II_files/image001.gif" v:shapes="Picture_x0020_45"><![endif]></span><span
    13921382style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    13931383
    … …  
    14151405 <v:imagedata src="RMCProfile-II_files/image088.png" o:title=""/>
    14161406</v:shape><![endif]--><![if !vml]><img border=0 width=480 height=400
    1417 src="RMCProfile-II_files/image019.gif" v:shapes="Picture_x0020_46"><![endif]></span><span
     1407src="RMCProfile-II_files/image002.gif" v:shapes="Picture_x0020_46"><![endif]></span><span
    14181408style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    14191409
    … …  
    14381428 <v:imagedata src="RMCProfile-II_files/image090.png" o:title=""/>
    14391429</v:shape><![endif]--><![if !vml]><img border=0 width=394 height=147
    1440 src="RMCProfile-II_files/image021.gif" v:shapes="Picture_x0020_47"><![endif]></span><span
     1430src="RMCProfile-II_files/image003.gif" v:shapes="Picture_x0020_47"><![endif]></span><span
    14411431style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    14421432
    … …  
    14461436fine.<o:p></o:p></span></p>
    14471437
    1448 <h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 3. Import SrTiO<sub>3
    1449 </sub>phase<o:p></o:p></span></h3>
     1438<h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 3. Import
     1439SrTiO<sub>3 </sub>phase<o:p></o:p></span></h3>
    14501440
    14511441<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>The
    14521442average structure of SrTiO<sub>3 </sub>is very simple. Space group I4/mcm, (or
    14531443Im-3m; a=5.48, c=7.75 with <span class=SpellE>Ti</span> at 0,0,0, <span
    1454 class=SpellE>Sr</span> at œ,0,Œ and O at 0,0,Œ <span
    1455 style='mso-spacerun:yes'> </span>and .241,.258,0. However, we will save time by
    1456 importing it from an old <span class=SpellE>gsas</span> experiment file which
    1457 has anisotropic thermal motion for the O atoms. </span>Use the <b
    1458 style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
    1459 mso-ascii-theme-font:minor-latin;mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:
    1460 minor-latin'>Import/Phase/from GSAS .EXP file</span></b> menu item to read the
    1461 phase information for <span style='mso-fareast-font-family:"Times New Roman"'>SrTiO<sub>3
    1462 </sub></span>into the current GSAS-II project. Other submenu items will read
    1463 phase information in other formats.<span style='mso-spacerun:yes'> 
    1464 </span>Because you used <span style='mso-fareast-font-family:Calibri;
    1465 mso-fareast-theme-font:minor-latin'>the </span><b style='mso-bidi-font-weight:
    1466 normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
    1467 minor-latin;mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin;
    1468 mso-hansi-theme-font:minor-latin'>Help/Download tutorial</span></b><span
     1444class=SpellE>Sr</span> at œ,0,Œ and O at 0,0,Œ<span style='mso-spacerun:yes'> 
     1445</span>and .241,.258,0. However, we will save time by importing it from an old <span
     1446class=SpellE>gsas</span> experiment file which has anisotropic thermal motion
     1447for the O atoms. </span>Use the <b style='mso-bidi-font-weight:normal'><span
     1448style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
     1449mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Import/Phase/from
     1450GSAS .EXP file</span></b> menu item to read the phase information for <span
     1451style='mso-fareast-font-family:"Times New Roman"'>SrTiO<sub>3 </sub></span>into
     1452the current GSAS-II project. Other submenu items will read phase information in
     1453other formats.<span style='mso-spacerun:yes'>  </span>Because you used <span
     1454style='mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin'>the </span><b
     1455style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
     1456mso-ascii-theme-font:minor-latin;mso-fareast-font-family:Calibri;mso-fareast-theme-font:
     1457minor-latin;mso-hansi-theme-font:minor-latin'>Help/Download tutorial</span></b><span
    14691458style='mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin'>
    14701459menu entry to open this page and downloaded the exercise files (recommended),
    1471 then the </span><span class=SpellE><b style='mso-bidi-font-weight:normal'><span
    1472 style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
    1473 mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin;mso-hansi-theme-font:
    1474 minor-latin'>RMCProfile</span></b></span><b style='mso-bidi-font-weight:normal'><span
    1475 style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
    1476 mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin;mso-hansi-theme-font:
    1477 minor-latin'>-II/data/...</span></b><span style='mso-fareast-font-family:Calibri;
    1478 mso-fareast-theme-font:minor-latin'> entry will bring you to the location where
    1479 the files have been downloaded. (It is also possible to download them manually
    1480 from <a
     1460then the </span><b style='mso-bidi-font-weight:normal'><span style='font-family:
     1461"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;mso-fareast-font-family:
     1462Calibri;mso-fareast-theme-font:minor-latin;mso-hansi-theme-font:minor-latin'>RMCProfile-II/data/...</span></b><span
     1463style='mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin'>
     1464entry will bring you to the location where the files have been downloaded. (It
     1465is also possible to download them manually from <a
    14811466href="https://subversion.xray.aps.anl.gov/pyGSAS/Tutorials/RMCProfile-II/data/">https://subversion.xray.aps.anl.gov/pyGSAS/Tutorials/RMCProfile-II/data/</a>.
    14821467In this case you will need to navigate to the download location manually.)
    … …  
    14991484normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
    15001485minor-latin;mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>SrTiO3</span></b>’;
    1501 NB: because of restrictions in <span class=SpellE>RMCProfile</span> it is
    1502 important that the phase name not have any spaces); press <b style='mso-bidi-font-weight:
    1503 normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
    1504 minor-latin;mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>OK</span></b>
     1486NB: because of restrictions in RMCProfile it is important that the phase name
     1487not have any spaces); press <b style='mso-bidi-font-weight:normal'><span
     1488style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
     1489mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>OK</span></b>
    15051490to continue. Next is the histogram selection window; this connects the phase to
    15061491the data so it can be used in subsequent calculations.</p>
    … …  
    15121497 <v:imagedata src="RMCProfile-II_files/image092.png" o:title=""/>
    15131498</v:shape><![endif]--><![if !vml]><img border=0 width=290 height=233
    1514 src="RMCProfile-II_files/image029.gif" v:shapes="Picture_x0020_48"><![endif]></span><span
     1499src="RMCProfile-II_files/image004.gif" v:shapes="Picture_x0020_48"><![endif]></span><span
    15151500style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    15161501
    … …  
    15291514 <v:imagedata src="RMCProfile-II_files/image094.png" o:title=""/>
    15301515</v:shape><![endif]--><![if !vml]><img border=0 width=478 height=244
    1531 src="RMCProfile-II_files/image077.gif" v:shapes="Picture_x0020_49"><![endif]></span><span
     1516src="RMCProfile-II_files/image005.gif" v:shapes="Picture_x0020_49"><![endif]></span><span
    15321517style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    15331518
    … …  
    15481533 <v:imagedata src="RMCProfile-II_files/image096.png" o:title=""/>
    15491534</v:shape><![endif]--><![if !vml]><img border=0 width=478 height=259
    1550 src="RMCProfile-II_files/image079.gif" v:shapes="Picture_x0020_50"><![endif]></span><span
     1535src="RMCProfile-II_files/image006.gif" v:shapes="Picture_x0020_50"><![endif]></span><span
    15511536style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    15521537
    15531538<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>Be
    1554 sure that “chebyschev-1” is used for the background function; <span
    1555 class=SpellE>RMCProfile</span> only recognizes that form to compute the
    1556 background for the diffraction pattern. Select </span><b style='mso-bidi-font-weight:
    1557 normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
    1558 minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
    1559 minor-latin;mso-bidi-theme-font:minor-latin'>6</span></b><span
     1539sure that “chebyschev-1” is used for the background function; RMCProfile only
     1540recognizes that form to compute the background for the diffraction pattern.
     1541Select </span><b style='mso-bidi-font-weight:normal'><span style='font-family:
     1542"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;mso-fareast-font-family:
     1543"Times New Roman";mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>6</span></b><span
    15601544style='mso-fareast-font-family:"Times New Roman"'> for the number of terms.<o:p></o:p></span></p>
    15611545
    … …  
    15741558mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:minor-latin;
    15751559mso-bidi-theme-font:minor-latin'>SrTiO3_5K</span></b><span style='mso-fareast-font-family:
    1576 "Times New Roman"'>”; do not use the phase name for this purpose because <span
    1577 class=SpellE>RMCProfile</span> will use that as the root for the many files it
    1578 creates. Also, you should create a new directory for this exercise while in
    1579 this dialog box; it will be rapidly filled up with <span class=SpellE>RMCProfile</span>
    1580 files which can lead to considerable confusion if mixed in with other files.
    1581 For Windows, after navigating to a suitable location, a new directory can be
    1582 made by a right mouse click and selecting “</span><b style='mso-bidi-font-weight:
    1583 normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
    1584 minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
    1585 minor-latin;mso-bidi-theme-font:minor-latin'>New/Folder</span></b><span
     1560"Times New Roman"'>”; do not use the phase name for this purpose because
     1561RMCProfile will use that as the root for the many files it creates. Also, you
     1562should create a new directory for this exercise while in this dialog box; it
     1563will be rapidly filled up with RMCProfile files which can lead to considerable
     1564confusion if mixed in with other files. For Windows, after navigating to a suitable
     1565location, a new directory can be made by a right mouse click and selecting “</span><b
     1566style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
     1567mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
     1568mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>New/Folder</span></b><span
    15861569style='mso-fareast-font-family:"Times New Roman"'>” from the popup menu. It
    15871570will appear with the name “New Folder”; change the name and select it (it will
    … …  
    15911574mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>OK</span></b><span
    15921575style='mso-fareast-font-family:"Times New Roman"'> to save the GSAS-II project
    1593 (SrTiO3_5K.gpx) and start the refinement. It will quickly converge to give a poor
    1594 <span class=SpellE>Rwp</span> (~44%) mostly because of mismatches in peak
     1576(SrTiO3_5K.gpx) and start the refinement. It will quickly converge to give a
     1577poor <span class=SpellE>Rwp</span> (~44%) mostly because of mismatches in peak
    15951578positions<o:p></o:p></span></p>
    15961579
    … …  
    16011584 <v:imagedata src="RMCProfile-II_files/image098.png" o:title=""/>
    16021585</v:shape><![endif]--><![if !vml]><img border=0 width=481 height=401
    1603 src="RMCProfile-II_files/image081.gif" v:shapes="Picture_x0020_51"><![endif]></span><span
     1586src="RMCProfile-II_files/image007.gif" v:shapes="Picture_x0020_51"><![endif]></span><span
    16041587style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    16051588
    … …  
    16231606<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    16241607mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_52" o:spid="_x0000_i1068"
    1625  type="#_x0000_t75" style='width:358.5pt;height:299.25pt;visibility:visible;
     1608 type="#_x0000_t75" style='width:357.75pt;height:299.25pt;visibility:visible;
    16261609 mso-wrap-style:square'>
    16271610 <v:imagedata src="RMCProfile-II_files/image100.png" o:title=""/>
    1628 </v:shape><![endif]--><![if !vml]><img border=0 width=478 height=399
    1629 src="RMCProfile-II_files/image083.gif" v:shapes="Picture_x0020_52"><![endif]></span><span
     1611</v:shape><![endif]--><![if !vml]><img border=0 width=477 height=399
     1612src="RMCProfile-II_files/image008.gif" v:shapes="Picture_x0020_52"><![endif]></span><span
    16301613style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    16311614
    … …  
    16911674mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>sig-2</span></b><span
    16921675style='mso-fareast-font-family:"Times New Roman"'> (normally not necessary, but
    1693 the available GEM instrument parameter file isn’t current). In any event, the
    1694 coefficients </span><span class=SpellE><b style='mso-bidi-font-weight:normal'><span
     1676the available GEM instrument parameter file isn’t current). In any event, the coefficients
     1677</span><span class=SpellE><b style='mso-bidi-font-weight:normal'><span
    16951678style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
    16961679mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:minor-latin;
    … …  
    17041687mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:minor-latin;
    17051688mso-bidi-theme-font:minor-latin'>sig-q</span></b><span style='mso-fareast-font-family:
    1706 "Times New Roman"'> must be zero since <span class=SpellE>RMCProfile</span>
    1707 V6.7.6 Beta Serial does not know how to use them in computing a powder profile.
    1708 <o:p></o:p></span></p>
     1689"Times New Roman"'> must be zero since RMCProfile V6.7.6 Beta Serial does not
     1690know how to use them in computing a powder profile. <o:p></o:p></span></p>
    17091691
    17101692<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>Do </span><b
    … …  
    17361718 <v:imagedata src="RMCProfile-II_files/image009.png" o:title=""/>
    17371719</v:shape><![endif]--><![if !vml]><img border=0 width=481 height=151
    1738 src="RMCProfile-II_files/image085.gif" v:shapes="Picture_x0020_53"><![endif]></span><span
     1720src="RMCProfile-II_files/image010.gif" v:shapes="Picture_x0020_53"><![endif]></span><span
    17391721style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    17401722
    17411723<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    1742 mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_55" o:spid="_x0000_i1066"
    1743  type="#_x0000_t75" style='width:5in;height:300pt;visibility:visible;
    1744  mso-wrap-style:square'>
     1724mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="_x0000_i1066" type="#_x0000_t75"
     1725 style='width:5in;height:300pt;visibility:visible;mso-wrap-style:square'>
    17451726 <v:imagedata src="RMCProfile-II_files/image011.png" o:title=""/>
    17461727</v:shape><![endif]--><![if !vml]><img border=0 width=480 height=400
    1747 src="RMCProfile-II_files/image087.gif" v:shapes="Picture_x0020_55"><![endif]></span><span
     1728src="RMCProfile-II_files/image012.gif" v:shapes="_x0000_i1066"><![endif]></span><span
    17481729style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    17491730
    … …  
    17631744showing the 50% ellipsoid surfaces (very small!)<o:p></o:p></span></p>
    17641745
    1765 <p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>2)
    1766 Double click the empty upper left box in the </span><b style='mso-bidi-font-weight:
     1746<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>2) Double
     1747click the empty upper left box in the </span><b style='mso-bidi-font-weight:
    17671748normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
    17681749minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
    … …  
    18301811 <v:imagedata src="RMCProfile-II_files/image013.png" o:title=""/>
    18311812</v:shape><![endif]--><![if !vml]><img border=0 width=624 height=520
    1832 src="RMCProfile-II_files/image089.gif" v:shapes="Picture_x0020_56"><![endif]></span><span
     1813src="RMCProfile-II_files/image014.gif" v:shapes="Picture_x0020_56"><![endif]></span><span
    18331814style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    18341815
    … …  
    18401821additional tilting as well that leads to a disk-like shape to the axial O-atoms
    18411822compared to the others. Next we will explore this with <span class=GramE>a</span>
    1842 <span class=SpellE>RMCProfile</span> simulation. To keep this drawing, you may want
    1843 to save the GSAS-II project.<o:p></o:p></span></p>
     1823RMCProfile simulation. To keep this drawing, you may want to save the GSAS-II
     1824project.<o:p></o:p></span></p>
    18441825
    18451826<h2><span style='mso-fareast-font-family:"Times New Roman"'>Reverse Monte Carlo
    … …  
    18511832mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:minor-latin;
    18521833mso-bidi-theme-font:minor-latin'>Phases/SrTiO3/RMC</span></b><span
    1853 style='mso-fareast-font-family:"Times New Roman"'> tab; if rmcprofile.exe is
    1854 within the GSASII directory the data window will show<o:p></o:p></span></p>
     1834style='mso-fareast-font-family:"Times New Roman"'> tab; if rmcprofile.exe is within
     1835the GSASII directory the data window will show<o:p></o:p></span></p>
    18551836
    18561837<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    … …  
    18601841 <v:imagedata src="RMCProfile-II_files/image093.png" o:title=""/>
    18611842</v:shape><![endif]--><![if !vml]><img border=0 width=481 height=320
    1862 src="RMCProfile-II_files/image091.gif" v:shapes="Picture_x0020_57"><![endif]></span><span
     1843src="RMCProfile-II_files/image015.gif" v:shapes="Picture_x0020_57"><![endif]></span><span
    18631844style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    18641845
    … …  
    18661847
    18671848<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>At
    1868 the top is a radio button selection for </span><span class=SpellE><b
    1869 style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
    1870 mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
    1871 mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>RMCProfile</span></b></span><span
     1849the top is a radio button selection for </span><b style='mso-bidi-font-weight:
     1850normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
     1851minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
     1852minor-latin;mso-bidi-theme-font:minor-latin'>RMCProfile</span></b><span
    18721853style='mso-fareast-font-family:"Times New Roman"'> and </span><span
    18731854class=SpellE><b style='mso-bidi-font-weight:normal'><span style='font-family:
    … …  
    18751856"Times New Roman";mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>fullrmc</span></b></span><span
    18761857style='mso-fareast-font-family:"Times New Roman"'>. The latter is an
    1877 alternative big box modeling program (not working – under development); <span
    1878 class=SpellE>RMCProfile</span> is selected by default and all below are its
    1879 setup controls. There are four major sections (metadata, major controls,
    1880 restraints &amp; constraints and data controls); we will work through each of
    1881 these in turn. The information you enter here is retained in the GSAS-II
    1882 project so you can easily try alternative setups without having to enter
    1883 everything over again. <o:p></o:p></span></p>
     1858alternative big box modeling program (not working – under development);
     1859RMCProfile is selected by default and all below are its setup controls. There
     1860are four major sections (metadata, major controls, restraints &amp; constraints
     1861and data controls); we will work through each of these in turn. The information
     1862you enter here is retained in the GSAS-II project so you can easily try
     1863alternative setups without having to enter everything over again. <o:p></o:p></span></p>
    18841864
    18851865<h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 1. Set
    … …  
    18871867
    18881868<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>The
    1889 entries here are for your convenience; there is no explicit use made of any of
    1890 these, but they will appear in some of the output files from <span
    1891 class=SpellE>RMCProfile</span> and of course will show here on subsequent views
    1892 of this window. Fill out as many of them as you see fit. I entered some things
    1893 for each as the defaults are somewhat nonsensical.<o:p></o:p></span></p>
     1869entries here are for your convenience; there is no explicit use made of any of these,
     1870but they will appear in some of the output files from RMCProfile and of course
     1871will show here on subsequent views of this window. Fill out as many of them as
     1872you see fit. I entered some things for each as the defaults are somewhat
     1873nonsensical.<o:p></o:p></span></p>
    18941874
    18951875<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    … …  
    18991879 <v:imagedata src="RMCProfile-II_files/image097.png" o:title=""/>
    19001880</v:shape><![endif]--><![if !vml]><img border=0 width=480 height=320
    1901 src="RMCProfile-II_files/image095.gif" v:shapes="Picture_x0020_58"><![endif]></span><span
     1881src="RMCProfile-II_files/image016.gif" v:shapes="Picture_x0020_58"><![endif]></span><span
    19021882style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    19031883
    … …  
    19151895minor-latin;mso-bidi-theme-font:minor-latin'>1</span></b><span
    19161896style='mso-fareast-font-family:"Times New Roman"'> minute. At each save time a
    1917 number of files are written by <span class=SpellE>RMCProfile</span>; these can
    1918 be viewed by using the Operations/View command (more about this later – don’t
    1919 bother trying it now, there is nothing to see). For the purposes of this
    1920 tutorial leave them at their defaults. <o:p></o:p></span></p>
     1897number of files are written by RMCProfile; these can be viewed by using the
     1898Operations/View command (more about this later – don’t bother trying it now,
     1899there is nothing to see). For the purposes of this tutorial leave them at their
     1900defaults. <o:p></o:p></span></p>
    19211901
    19221902<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>The
    1923 big box model used by <span class=SpellE>RMCProfile</span> is described as
    1924 multiples of the unit cell axes. In this case we want a 6x6x4 box so enter </span><b
    1925 style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
    1926 mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
    1927 mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>6</span></b><span
     1903big box model used by RMCProfile is described as multiples of the unit cell
     1904axes. In this case we want a 6x6x4 box so enter </span><b style='mso-bidi-font-weight:
     1905normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
     1906minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
     1907minor-latin;mso-bidi-theme-font:minor-latin'>6</span></b><span
    19281908style='mso-fareast-font-family:"Times New Roman"'> for each of </span><b
    19291909style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
    … …  
    19611941isn’t appropriate; if changed the window will repaint updating various entries
    19621942possibly resetting some entries to defaults. I suggest you decide the order now
    1963 and then don’t change it later. Change it to <span class=SpellE>Sr</span>, <span
    1964 class=SpellE>Ti</span>, O; the <span class=SpellE>windo</span> will repaint
     1943and then don’t change it later. Change it to </span><span class=SpellE><b
     1944style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
     1945mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
     1946mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Sr</span></b></span><span
     1947style='mso-fareast-font-family:"Times New Roman"'>, </span><span class=SpellE><b
     1948style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
     1949mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
     1950mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Ti</span></b></span><span
     1951style='mso-fareast-font-family:"Times New Roman"'>, </span><b style='mso-bidi-font-weight:
     1952normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
     1953minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
     1954minor-latin;mso-bidi-theme-font:minor-latin'>O</span></b><span
     1955style='mso-fareast-font-family:"Times New Roman"'>; the window will repaint
    19651956each time. Set the maximum shift for <span class=SpellE>Sr</span> and <span
    19661957class=SpellE>Ti</span> to be </span><b style='mso-bidi-font-weight:normal'><span
    … …  
    19731964<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    19741965mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_59" o:spid="_x0000_i1062"
    1975  type="#_x0000_t75" style='width:359.25pt;height:239.25pt;visibility:visible;
     1966 type="#_x0000_t75" style='width:5in;height:239.25pt;visibility:visible;
    19761967 mso-wrap-style:square'>
    19771968 <v:imagedata src="RMCProfile-II_files/image101.png" o:title=""/>
    1978 </v:shape><![endif]--><![if !vml]><img border=0 width=479 height=319
    1979 src="RMCProfile-II_files/image099.gif" v:shapes="Picture_x0020_59"><![endif]></span><span
     1969</v:shape><![endif]--><![if !vml]><img border=0 width=480 height=319
     1970src="RMCProfile-II_files/image018.gif" v:shapes="Picture_x0020_59"><![endif]></span><span
    19801971style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    19811972
    … …  
    19881979
    19891980<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>Next
    1990 is to set the “Hard” minimum atom-atom separation and the allowed search rage for
    1991 each of 6 pairs of atom types. Possible values for this table can be obtained
    1992 in GSAS-II by computing bond lengths. Select the </span><b style='mso-bidi-font-weight:
    1993 normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
    1994 minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
    1995 minor-latin;mso-bidi-theme-font:minor-latin'>Atoms</span></b><span
     1981is to set the “Hard” minimum atom-atom separation and the allowed search rage
     1982for each of 6 pairs of atom types. Possible values for this table can be
     1983obtained in GSAS-II by computing bond lengths. Select the </span><b
     1984style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
     1985mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
     1986mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Atoms</span></b><span
    19961987style='mso-fareast-font-family:"Times New Roman"'> tab and then select all
    19971988atoms by double clicking on the empty upper left box in the table.<o:p></o:p></span></p>
    … …  
    19991990<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    20001991mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_60" o:spid="_x0000_i1061"
    2001  type="#_x0000_t75" style='width:362.25pt;height:116.25pt;visibility:visible;
     1992 type="#_x0000_t75" style='width:361.5pt;height:116.25pt;visibility:visible;
    20021993 mso-wrap-style:square'>
    20031994 <v:imagedata src="RMCProfile-II_files/image020.png" o:title=""/>
    2004 </v:shape><![endif]--><![if !vml]><img border=0 width=483 height=155
    2005 src="RMCProfile-II_files/image102.gif" v:shapes="Picture_x0020_60"><![endif]></span><span
     1995</v:shape><![endif]--><![if !vml]><img border=0 width=482 height=155
     1996src="RMCProfile-II_files/image022.gif" v:shapes="Picture_x0020_60"><![endif]></span><span
    20061997style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    20071998
    … …  
    20192010 <v:imagedata src="RMCProfile-II_files/image023.png" o:title=""/>
    20202011</v:shape><![endif]--><![if !vml]><img border=0 width=275 height=262
    2021 src="RMCProfile-II_files/image103.gif" v:shapes="Picture_x0020_61"><![endif]></span><span
     2012src="RMCProfile-II_files/image024.gif" v:shapes="Picture_x0020_61"><![endif]></span><span
    20222013style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    20232014
    … …  
    20732064 <v:imagedata src="RMCProfile-II_files/image025.png" o:title=""/>
    20742065</v:shape><![endif]--><![if !vml]><img border=0 width=479 height=234
    2075 src="RMCProfile-II_files/image104.gif" v:shapes="Picture_x0020_62"><![endif]></span><span
     2066src="RMCProfile-II_files/image026.gif" v:shapes="Picture_x0020_62"><![endif]></span><span
    20762067style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    20772068
    … …  
    20842075<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>We
    20852076will be using three different types of SrTiO<sub>3</sub> data for the fitting
    2086 by <span class=SpellE>RMCProfile</span>. The first is the selection of the
    2087 powder pattern (“Bragg”) for processing. This is taken from the PWDR entries in
    2088 the GSAS-II project and accessed from the pulldown; there is only one “</span><b
    2089 style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
    2090 mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
    2091 mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>PWDR gem05984.gss
    2092 Bank 3</span></b><span style='mso-fareast-font-family:"Times New Roman"'>” that
    2093 was used earlier in your Rietveld refinement of SrTiO<sub>3</sub>. If you had
    2094 used multiple banks in the Rietveld refinement, all would be shown in the
    2095 pulldown, but only one can be selected. Set the weight to </span><b
    2096 style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
    2097 mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
    2098 mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>0.5</span></b><span
    2099 style='mso-fareast-font-family:"Times New Roman"'> (NB: smaller numbers means a
    2100 heavier weight).<o:p></o:p></span></p>
     2077by RMCProfile. The first is the selection of the powder pattern (“Bragg”) for
     2078processing. This is taken from the PWDR entries in the GSAS-II project and
     2079accessed from the pulldown; there is only one “</span><b style='mso-bidi-font-weight:
     2080normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
     2081minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
     2082minor-latin;mso-bidi-theme-font:minor-latin'>PWDR gem05984.gss Bank 3</span></b><span
     2083style='mso-fareast-font-family:"Times New Roman"'>” that was used earlier in
     2084your Rietveld refinement of SrTiO<sub>3</sub>. If you had used multiple banks
     2085in the Rietveld refinement, all would be shown in the pulldown, but only one
     2086can be selected. Set the weight to </span><b style='mso-bidi-font-weight:normal'><span
     2087style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
     2088mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:minor-latin;
     2089mso-bidi-theme-font:minor-latin'>0.5</span></b><span style='mso-fareast-font-family:
     2090"Times New Roman"'> (NB: smaller numbers means a heavier weight).<o:p></o:p></span></p>
    21012091
    21022092<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>Next
    … …  
    21162106style='mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin'>
    21172107menu entry to open this page and downloaded the exercise files (recommended),
    2118 then the </span><span class=SpellE><b style='mso-bidi-font-weight:normal'><span
    2119 style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
    2120 mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin;mso-hansi-theme-font:
    2121 minor-latin'>RMCProfile</span></b></span><b style='mso-bidi-font-weight:normal'><span
    2122 style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
    2123 mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin;mso-hansi-theme-font:
    2124 minor-latin'>-I/data/...</span></b><span style='mso-fareast-font-family:Calibri;
    2125 mso-fareast-theme-font:minor-latin'> entry will bring you to the location where
    2126 the files have been downloaded. (It is also possible to download them manually
    2127 from <a
    2128 href="https://subversion.xray.aps.anl.gov/pyGSAS/Tutorials/RMCProfile-I/data/">https://subversion.xray.aps.anl.gov/pyGSAS/Tutorials/RMCProfile-I/data/</a>.
     2108then the </span><b style='mso-bidi-font-weight:normal'><span style='font-family:
     2109"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;mso-fareast-font-family:
     2110Calibri;mso-fareast-theme-font:minor-latin;mso-hansi-theme-font:minor-latin'>RMCProfile-II/data/...</span></b><span
     2111style='mso-fareast-font-family:Calibri;mso-fareast-theme-font:minor-latin'>
     2112entry will bring you to the location where the files have been downloaded. (It
     2113is also possible to download them manually from <a
     2114href="https://subversion.xray.aps.anl.gov/pyGSAS/Tutorials/RMCProfile-II/data/">https://subversion.xray.aps.anl.gov/pyGSAS/Tutorials/RMCProfile-II/data/</a>.
    21292115In this case you will need to navigate to the download location manually.)<o:p></o:p></span></p>
    21302116
    … …  
    21382124 <v:imagedata src="RMCProfile-II_files/image105.png" o:title=""/>
    21392125</v:shape><![endif]--><![if !vml]><img border=0 width=478 height=194
    2140 src="RMCProfile-II_files/image106.gif" v:shapes="Picture_x0020_63"><![endif]></span><span
     2126src="RMCProfile-II_files/image027.gif" v:shapes="Picture_x0020_63"><![endif]></span><span
    21412127style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    21422128
    … …  
    21462132mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>srtio3_wk_5k_rmc.gr</span></b><span
    21472133style='mso-fareast-font-family:"Times New Roman"'>; it will be copied from this
    2148 location to your working directory for this tutorial (<span class=SpellE>RMCProfile</span>
    2149 requires all its files to be local). The window will be redrawn showing the new
    2150 entry; the weight is fine.<o:p></o:p></span></p>
     2134location to your working directory for this tutorial (RMCProfile requires all
     2135its files to be local). The window will be redrawn showing the new entry; the
     2136weight is fine.<o:p></o:p></span></p>
    21512137
    21522138<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    … …  
    21562142 <v:imagedata src="RMCProfile-II_files/image107.png" o:title=""/>
    21572143</v:shape><![endif]--><![if !vml]><img border=0 width=481 height=235
    2158 src="RMCProfile-II_files/image108.gif" v:shapes="Picture_x0020_64"><![endif]></span><span
     2144src="RMCProfile-II_files/image028.gif" v:shapes="Picture_x0020_64"><![endif]></span><span
    21592145style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    21602146
    … …  
    21732159 <v:imagedata src="RMCProfile-II_files/image109.png" o:title=""/>
    21742160</v:shape><![endif]--><![if !vml]><img border=0 width=479 height=194
    2175 src="RMCProfile-II_files/image110.gif" v:shapes="Picture_x0020_65"><![endif]></span><span
     2161src="RMCProfile-II_files/image030.gif" v:shapes="Picture_x0020_65"><![endif]></span><span
    21762162style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    21772163
    … …  
    21892175 <v:imagedata src="RMCProfile-II_files/image111.png" o:title=""/>
    21902176</v:shape><![endif]--><![if !vml]><img border=0 width=479 height=234
    2191 src="RMCProfile-II_files/image112.gif" v:shapes="Picture_x0020_70"><![endif]></span><span
     2177src="RMCProfile-II_files/image031.gif" v:shapes="Picture_x0020_70"><![endif]></span><span
    21922178style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    21932179
    … …  
    22012187 <v:imagedata src="RMCProfile-II_files/image113.png" o:title=""/>
    22022188</v:shape><![endif]--><![if !vml]><img border=0 width=479 height=175
    2203 src="RMCProfile-II_files/image114.gif" v:shapes="Picture_x0020_67"><![endif]></span><span
    2204 style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    2205 
    2206 <h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 5. Setup <span
    2207 class=SpellE>RMCProfile</span> files<o:p></o:p></span></h3>
     2189src="RMCProfile-II_files/image032.gif" v:shapes="Picture_x0020_67"><![endif]></span><span
     2190style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
     2191
     2192<h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 5. Setup
     2193RMCProfile files<o:p></o:p></span></h3>
    22082194
    22092195<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>You
    2210 are now ready to setup the <span class=SpellE>RMCProfile</span> input files<span
    2211 class=GramE>..</span> Do </span><b style='mso-bidi-font-weight:normal'><span
    2212 style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
    2213 mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:minor-latin;
    2214 mso-bidi-theme-font:minor-latin'>Operations/Setup RMC</span></b><span
    2215 style='mso-fareast-font-family:"Times New Roman"'> from the menu; the console
    2216 should report that files were written<o:p></o:p></span></p>
     2196are now ready to setup the RMCProfile input files<span class=GramE>..</span> Do
     2197</span><b style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
     2198mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
     2199mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Operations/Setup
     2200RMC</span></b><span style='mso-fareast-font-family:"Times New Roman"'> from the
     2201menu; the console should report that files were written<o:p></o:p></span></p>
    22172202
    22182203<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    … …  
    22222207 <v:imagedata src="RMCProfile-II_files/image115.png" o:title=""/>
    22232208</v:shape><![endif]--><![if !vml]><img border=0 width=285 height=107
    2224 src="RMCProfile-II_files/image116.gif" v:shapes="Picture_x0020_68"><![endif]></span><span
     2209src="RMCProfile-II_files/image033.gif" v:shapes="Picture_x0020_68"><![endif]></span><span
    22252210style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    22262211
    … …  
    22312216<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    22322217mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_69" o:spid="_x0000_i1052"
    2233  type="#_x0000_t75" style='width:360.75pt;height:164.25pt;visibility:visible;
     2218 type="#_x0000_t75" style='width:5in;height:164.25pt;visibility:visible;
    22342219 mso-wrap-style:square'>
    22352220 <v:imagedata src="RMCProfile-II_files/image117.png" o:title=""/>
    2236 </v:shape><![endif]--><![if !vml]><img border=0 width=481 height=219
    2237 src="RMCProfile-II_files/image118.gif" v:shapes="Picture_x0020_69"><![endif]></span><span
     2221</v:shape><![endif]--><![if !vml]><img border=0 width=480 height=219
     2222src="RMCProfile-II_files/image034.gif" v:shapes="Picture_x0020_69"><![endif]></span><span
    22382223style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    22392224
    22402225<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>These
    2241 text files contain data needed by <span class=SpellE>RMCProfile</span> for the
    2242 fitting of SF6. They are:<o:p></o:p></span></p>
     2226text files contain data needed by RMCProfile for the fitting of SF6. They are:<o:p></o:p></span></p>
    22432227
    22442228<p class=MsoNormal><b style='mso-bidi-font-weight:normal'><span
    … …  
    22542238<p class=MsoNormal><b style='mso-bidi-font-weight:normal'><span
    22552239style='mso-fareast-font-family:"Times New Roman"'>SrTiO3.dat</span></b><span
    2256 style='mso-fareast-font-family:"Times New Roman"'> – the <span class=SpellE>RMCProfile</span>
    2257 controls file; described in full in the <span class=SpellE>RMCProfile</span>
    2258 User Manual. It can be edited if need be, but remember it is rewritten each
    2259 time Operations/Setup RMC is done.<o:p></o:p></span></p>
     2240style='mso-fareast-font-family:"Times New Roman"'> – the RMCProfile controls
     2241file; described in full in the RMCProfile User Manual. It can be edited if need
     2242be, but remember it is rewritten each time Operations/Setup RMC is done.<o:p></o:p></span></p>
    22602243
    22612244<p class=MsoNormal><b style='mso-bidi-font-weight:normal'><span
    … …  
    22632246style='mso-fareast-font-family:"Times New Roman"'> – the instrument parameter
    22642247coefficients for the neutron TOF peak shape function used by GSAS-II and
    2265 implemented in <span class=SpellE>RMCProfile</span> for computing the Bragg
    2266 pattern.<o:p></o:p></span></p>
     2248implemented in RMCProfile for computing the Bragg pattern.<o:p></o:p></span></p>
    22672249
    22682250<p class=MsoNormal><b style='mso-bidi-font-weight:normal'><span
    … …  
    22722254unless the X-axis, Y-axis, or Z-axis lattice multipliers are changed. Most
    22732255important is that it will contain the set of big box atom positions as updated
    2274 by <span class=SpellE>RMCProfile</span> according to the Save interval (every 1
    2275 min in this case).<o:p></o:p></span></p>
     2256by RMCProfile according to the Save interval (every 1 min in this case).<o:p></o:p></span></p>
    22762257
    22772258<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>You
    2278 are now ready to run <span class=SpellE>RMCProfile</span>.<o:p></o:p></span></p>
    2279 
    2280 <h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 6. Run <span
    2281 class=SpellE>RMCProfile</span><o:p></o:p></span></h3>
     2259are now ready to run RMCProfile.<o:p></o:p></span></p>
     2260
     2261<h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 6. Run
     2262RMCProfile<o:p></o:p></span></h3>
    22822263
    22832264<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>To
    2284 run <span class=SpellE>RMCProfile</span> from inside GSAS-II, do </span><b
    2285 style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
    2286 mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
    2287 mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Operations/Execute</span></b><span
     2265run RMCProfile from inside GSAS-II, do </span><b style='mso-bidi-font-weight:
     2266normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
     2267minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
     2268minor-latin;mso-bidi-theme-font:minor-latin'>Operations/Execute</span></b><span
    22882269style='mso-fareast-font-family:"Times New Roman"'>. You will first see a “nag”
    2289 note asking you to cite the publication describing <span class=SpellE>RMCProfile</span>;
    2290 press </span><b style='mso-bidi-font-weight:normal'><span style='font-family:
    2291 "Calibri",sans-serif;mso-ascii-theme-font:minor-latin;mso-fareast-font-family:
    2292 "Times New Roman";mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>OK</span></b><span
     2270note asking you to cite the publication describing RMCProfile; press </span><b
     2271style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
     2272mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
     2273mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>OK</span></b><span
    22932274style='mso-fareast-font-family:"Times New Roman"'>.<o:p></o:p></span></p>
    22942275
    … …  
    22982279used and <span class=GramE>Last</span> saved. Once the latter is nonzero you
    22992280can view intermediate results to see its progress. It also shows the chi^2 for
    2300 each of the contributing data sets; these start in the 5-300 range and will quickly
    2301 drop in the initial stages of the run. Note that you can exit GSAS-II and <span
    2302 class=SpellE>RMCProfile</span> will continue running. After <span class=SpellE>RMCProfile</span>
    2303 finishes note that the project directory now has ~30 files many of which are
    2304 just temporary ones created by <span class=SpellE>RMCProfile</span>. We will be
    2305 looking at just the *.csv files and the SrTiO3.rmcf6 file; the latter contains
    2306 the last atom configuration acceptable by <span class=SpellE>RMCProfile</span>
    2307 thus representing a best disordered model.<o:p></o:p></span></p>
     2281each of the contributing data sets; these start in the 5-300 range and will
     2282quickly drop in the initial stages of the run. Note that you can exit GSAS-II
     2283and RMCProfile will continue running. After RMCProfile finishes note that the
     2284project directory now has ~30 files many of which are just temporary ones
     2285created by RMCProfile. We will be looking at just the *.csv files and the
     2286SrTiO3.rmcf6 file; the latter contains the last atom configuration acceptable
     2287by RMCProfile thus representing a best disordered model.<o:p></o:p></span></p>
    23082288
    23092289<h3><span style='mso-fareast-font-family:"Times New Roman"'>A note about
    … …  
    23112291
    23122292<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>The
    2313 choice of weights for <span class=SpellE>RMCProfile</span> may seem to be
    2314 arbitrary in these exercises, but I have selected them so that each of the
    2315 chi^2 values converge to be roughly equal and somewhere just above unity. This
    2316 selection generally gives the best performance in the reverse Monte Carlo calculation
    2317 and requires some “trial &amp; effort” in selecting the values. If one of the
    2318 chi^2 values is too large (&gt;&gt;1, i.e. weight too small) at convergence,
    2319 then adjustments in the structure will have been dominated by moves that lower
    2320 that chi^2 sometimes at the expense of others. Conversely, if one chi^2 is too
    2321 small (&gt;&gt;1, i.e. weight too large) then moves will tend to satisfy the
    2322 others and there will be little sensitivity to that data set. In this case my
    2323 chosen weights have yielded 1.003 for the Bragg, 2.980 for the G(R) “<span
    2324 class=SpellE>Expt</span> 1” and 1.899 for the F(Q) “<span class=SpellE>Expt</span>
    2325 2” data sets; this is essentially ideal. If they vary by more than an order of
    2326 magnitude or are less than unity, you should adjust the weights.<o:p></o:p></span></p>
     2293choice of weights for RMCProfile may seem to be arbitrary in these exercises,
     2294but I have selected them so that each of the chi^2 values converge to be
     2295roughly equal and somewhere just above unity. This selection generally gives
     2296the best performance in the reverse Monte Carlo calculation and requires some
     2297“trial &amp; effort” in selecting the values. If one of the chi^2 values is too
     2298large (&gt;&gt;1, i.e. weight too small) at convergence, then adjustments in
     2299the structure will have been dominated by moves that lower that chi^2 sometimes
     2300at the expense of others. Conversely, if one chi^2 is too small (&gt;&gt;1,
     2301i.e. weight too large) then moves will tend to satisfy the others and there
     2302will be little sensitivity to that data set. In this case my chosen weights
     2303have yielded 1.003 for the Bragg, 2.980 for the G(R) “<span class=SpellE>Expt</span>
     23041” and 1.899 for the F(Q) “<span class=SpellE>Expt</span> 2” data sets; this is
     2305essentially ideal. If they vary by more than an order of magnitude or are less
     2306than unity, you should adjust the weights.<o:p></o:p></span></p>
    23272307
    23282308<h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 7. Viewing
    2329 results from <span class=SpellE>RMCProfile</span><o:p></o:p></span></h3>
     2309results from RMCProfile<o:p></o:p></span></h3>
    23302310
    23312311<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>Do </span><b
    … …  
    23432323 <v:imagedata src="RMCProfile-II_files/image119.png" o:title=""/>
    23442324</v:shape><![endif]--><![if !vml]><img border=0 width=481 height=166
    2345 src="RMCProfile-II_files/image120.gif" v:shapes="Picture_x0020_71"><![endif]></span><span
     2325src="RMCProfile-II_files/image035.gif" v:shapes="Picture_x0020_71"><![endif]></span><span
    23462326style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    23472327
    … …  
    23502330from the GSAS-II project file. Select any one of them – it doesn’t matter. All
    23512331of them will be read and their contents displayed as individual plots. For
    2352 example the chi^2 plot shows the progress of the <span class=SpellE>RMCProfile</span>
    2353 fit<o:p></o:p></span></p>
     2332example the chi^2 plot shows the progress of the RMCProfile fit<o:p></o:p></span></p>
    23542333
    23552334<p class=MsoNormal><!--[if mso & !supportInlineShapes & supportFields]><span
    … …  
    23592338 id="Group_x0020_5" o:spid="_x0000_s1026" style='width:358.9pt;height:299.4pt;
    23602339 mso-position-horizontal-relative:char;mso-position-vertical-relative:line'
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    … …  
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    … …  
    39473928 <w:anchorlock/>
    39483929</v:group><![endif]--><![if !vml]><img width=479 height=399
    3949 src="RMCProfile-II_files/image123.gif" v:shapes="Group_x0020_5 Picture_x0020_2 Picture_x0020_3"><![endif]><!--[if mso & !supportInlineShapes & supportFields]><v:shape
     3930src="RMCProfile-II_files/image036.gif" v:shapes="Group_x0020_5 Picture_x0020_2 Picture_x0020_3"><![endif]><!--[if mso & !supportInlineShapes & supportFields]><v:shape
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    … …  
    39543935
    39553936<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>The
    3956 inset is the upper 3/4ths of the plot magnified; you can see that <span
    3957 class=SpellE>RMCProfile</span> is still improving the fit slowly even after 10
    3958 minutes of running.<o:p></o:p></span></p>
     3937inset is the upper 3/4ths of the plot magnified; you can see that RMCProfile is
     3938still improving the fit slowly even after 10 minutes of running.<o:p></o:p></span></p>
    39593939
    39603940<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    … …  
    39643944 <v:imagedata src="RMCProfile-II_files/image124.png" o:title=""/>
    39653945</v:shape><![endif]--><![if !vml]><img border=0 width=478 height=430
    3966 src="RMCProfile-II_files/image125.gif" v:shapes="Picture_x0020_75"><![endif]></span><span
     3946src="RMCProfile-II_files/image037.gif" v:shapes="Picture_x0020_75"><![endif]></span><span
    39673947style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    39683948
    … …  
    39703950G(R) partials plot shows the identity of each feature; because titanium has a
    39713951negative neutron scattering length the first sharp peak (1.93Å) is negative and
    3972 arises from <span class=SpellE>Ti</span>-O. The next one (2.74Å) is an exact overlap
    3973 of O-O and <span class=SpellE>Sr</span>-O distances. One can easily see other
    3974 peaks involving <span class=SpellE>Ti</span> as well as identify which atom
    3975 pairs contribute to every feature of the PDF. <span style='mso-no-proof:yes'>Comparing
    3976 the Bragg plot with the PWDR plot shows that the RMCProfile fit is very similar
    3977 to the Rietveld fit<o:p></o:p></span></span></p>
     3952arises from <span class=SpellE>Ti</span>-O. The next one (2.74Å) is an exact
     3953overlap of O-O and <span class=SpellE>Sr</span>-O distances. One can easily see
     3954other peaks involving <span class=SpellE>Ti</span> as well as identify which
     3955atom pairs contribute to every feature of the PDF. <span style='mso-no-proof:
     3956yes'>Comparing the Bragg plot with the PWDR plot shows that the RMCProfile fit
     3957is very similar to the Rietveld fit<o:p></o:p></span></span></p>
    39783958
    39793959<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    … …  
    39833963 <v:imagedata src="RMCProfile-II_files/image126.png" o:title=""/>
    39843964</v:shape><![endif]--><![if !vml]><img border=0 width=480 height=453
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     3965src="RMCProfile-II_files/image038.gif" v:shapes="Picture_x0020_77"><![endif]></span><span
    39863966style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    39873967
    … …  
    39953975<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    39963976mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_78" o:spid="_x0000_i1047"
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     3977 type="#_x0000_t75" style='width:5in;height:339pt;visibility:visible;
    39983978 mso-wrap-style:square'>
    39993979 <v:imagedata src="RMCProfile-II_files/image128.png" o:title=""/>
    4000 </v:shape><![endif]--><![if !vml]><img border=0 width=479 height=452
    4001 src="RMCProfile-II_files/image129.gif" v:shapes="Picture_x0020_78"><![endif]></span><span
     3980</v:shape><![endif]--><![if !vml]><img border=0 width=480 height=452
     3981src="RMCProfile-II_files/image039.gif" v:shapes="Picture_x0020_78"><![endif]></span><span
    40023982style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    40033983
    … …  
    40073987especially evident in the <span class=GramE>S(</span>Q) plot where the data is
    40083988less than the RMC calculated result. Both of these issues arise from faults in
    4009 the data processing. The scaling can be corrected in <span class=SpellE>RMCProfile</span>
    4010 but the peak offset must be fixed first.<o:p></o:p></span></p>
     3989the data processing. The scaling can be corrected in RMCProfile but the peak
     3990offset must be fixed first.<o:p></o:p></span></p>
    40113991
    40123992<h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 8. Fixing peak
    … …  
    40163996peak offset in this case arises from different diffractometer constants
    40173997(especially <span class=SpellE>difC</span>) used for the Rietveld refinement
    4018 and the processing for <span class=GramE>F(</span>Q) and G(R). To fix this one
     3998and the processing for <span class=GramE>F(</span>Q) and G(R). To fix this, one
    40193999must adjust <span class=SpellE>difC</span> and repeat the Rietveld refinement.
    40204000This shifts the lattice parameters and ultimately the size of the big box
    … …  
    40324012 <v:imagedata src="RMCProfile-II_files/image040.png" o:title=""/>
    40334013</v:shape><![endif]--><![if !vml]><img border=0 width=383 height=393
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    40354015style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    40364016
    … …  
    40484028<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
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    4053 </v:shape><![endif]--><![if !vml]><img border=0 width=480 height=451
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     4033</v:shape><![endif]--><![if !vml]><img border=0 width=480 height=452
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    40554035style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    40564036
    … …  
    40714051 <v:imagedata src="RMCProfile-II_files/image044.png" o:title=""/>
    40724052</v:shape><![endif]--><![if !vml]><img border=0 width=392 height=175
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     4053src="RMCProfile-II_files/image045.gif" v:shapes="Picture_x0020_81"><![endif]></span><span
    40744054style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    40754055
    … …  
    40964076
    40974077<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>Now
    4098 you have to repeat the <span class=SpellE>RMCProfile</span> run starting from a
    4099 fresh set of lattice parameters and atom positions. This requires a new
    4100 SrTiO3.rmc6f file. Select the </span><b style='mso-bidi-font-weight:normal'><span
    4101 style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
    4102 mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:minor-latin;
    4103 mso-bidi-theme-font:minor-latin'>SrTiO3/RMC</span></b><span style='mso-fareast-font-family:
    4104 "Times New Roman"'> tab<span style='mso-no-proof:yes'><!--[if gte vml 1]><v:shape
    4105  id="Picture_x0020_82" o:spid="_x0000_i1043" type="#_x0000_t75" style='width:357.75pt;
    4106  height:273.75pt;visibility:visible;mso-wrap-style:square'>
     4078you have to repeat the RMCProfile run starting from a fresh set of lattice
     4079parameters and atom positions. This requires a new SrTiO3.rmc6f file. Select
     4080the </span><b style='mso-bidi-font-weight:normal'><span style='font-family:
     4081"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;mso-fareast-font-family:
     4082"Times New Roman";mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>SrTiO3/RMC</span></b><span
     4083style='mso-fareast-font-family:"Times New Roman"'> tab<span style='mso-no-proof:
     4084yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_82" o:spid="_x0000_i1043"
     4085 type="#_x0000_t75" style='width:357.75pt;height:273.75pt;visibility:visible;
     4086 mso-wrap-style:square'>
    41074087 <v:imagedata src="RMCProfile-II_files/image046.png" o:title=""/>
    41084088</v:shape><![endif]--><![if !vml]><img border=0 width=477 height=365
    4109 src="RMCProfile-II_files/image135.gif" v:shapes="Picture_x0020_82"><![endif]></span><o:p></o:p></span></p>
     4089src="RMCProfile-II_files/image047.gif" v:shapes="Picture_x0020_82"><![endif]></span><o:p></o:p></span></p>
    41104090
    41114091<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>Pick
    … …  
    41514131 <v:imagedata src="RMCProfile-II_files/image048.png" o:title=""/>
    41524132</v:shape><![endif]--><![if !vml]><img border=0 width=399 height=114
    4153 src="RMCProfile-II_files/image136.gif" v:shapes="Picture_x0020_83"><![endif]></span><o:p></o:p></span></p>
     4133src="RMCProfile-II_files/image049.gif" v:shapes="Picture_x0020_83"><![endif]></span><o:p></o:p></span></p>
    41544134
    41554135<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>Then
    … …  
    41614141mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
    41624142mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Ok</span></b><span
    4163 style='mso-fareast-font-family:"Times New Roman"'> to the nag note) to run <span
    4164 class=SpellE>RMCProfile</span>. As it runs it will report on its console the
    4165 scale factors for each <span class=SpellE>Expt</span> data set: ~1.14 for G(R) “<span
    4166 class=SpellE>Expt</span> 1” and ~1.21 for <span class=GramE>F(</span>Q) “<span
    4167 class=SpellE>Expt</span> 2”. When completed, the chi^2 values for G(R) (0.6513
    4168 vs 2.980) and <span class=GramE>F(</span>Q) (0.1258 vs 1.899) are much improved
    4169 while the Bragg fit is essentially unchanged (0.9684 vs 1.003). To see the
    4170 result do </span><b style='mso-bidi-font-weight:normal'><span style='font-family:
    4171 "Calibri",sans-serif;mso-ascii-theme-font:minor-latin;mso-fareast-font-family:
    4172 "Times New Roman";mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Operations/View</span></b><span
     4143style='mso-fareast-font-family:"Times New Roman"'> to the nag note) to run
     4144RMCProfile. As it runs it will report on its console the scale factors for each
     4145<span class=SpellE>Expt</span> data set: ~1.14 for G(R) “<span class=SpellE>Expt</span>
     41461” and ~1.21 for <span class=GramE>F(</span>Q) “<span class=SpellE>Expt</span>
     41472”. When completed, the chi^2 values for G(R) (0.6513 vs 2.980) and <span
     4148class=GramE>F(</span>Q) (0.1258 vs 1.899) are much improved while the Bragg fit
     4149is essentially unchanged (0.9684 vs 1.003). To see the result do </span><b
     4150style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
     4151mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
     4152mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Operations/View</span></b><span
    41734153style='mso-fareast-font-family:"Times New Roman"'>; the peaks in the </span><b
    41744154style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
    … …  
    41814161<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    41824162mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_84" o:spid="_x0000_i1041"
    4183  type="#_x0000_t75" style='width:359.25pt;height:336.75pt;visibility:visible;
     4163 type="#_x0000_t75" style='width:5in;height:336.75pt;visibility:visible;
    41844164 mso-wrap-style:square'>
    41854165 <v:imagedata src="RMCProfile-II_files/image050.png" o:title=""/>
    4186 </v:shape><![endif]--><![if !vml]><img border=0 width=479 height=449
    4187 src="RMCProfile-II_files/image137.gif" v:shapes="Picture_x0020_84"><![endif]></span><span
     4166</v:shape><![endif]--><![if !vml]><img border=0 width=480 height=449
     4167src="RMCProfile-II_files/image051.gif" v:shapes="Picture_x0020_84"><![endif]></span><span
    41884168style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    41894169
    … …  
    42144194mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Operations/Setup
    42154195RMC</span></b><span style='mso-fareast-font-family:"Times New Roman"'> to
    4216 update the <span class=SpellE>RMCProfile</span> files and then do </span><b
    4217 style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
    4218 mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
    4219 mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>Operations/Execute</span></b><span
     4196update the RMCProfile files and then do </span><b style='mso-bidi-font-weight:
     4197normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
     4198minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
     4199minor-latin;mso-bidi-theme-font:minor-latin'>Operations/Execute</span></b><span
    42204200style='mso-fareast-font-family:"Times New Roman"'> again for another 10min. My
    42214201result gave Bragg chi^2 = 0.9619, G(R) chi^2 =1.769 and <span class=GramE>F(</span>Q)
    … …  
    42314211normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
    42324212minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
    4233 minor-latin;mso-bidi-theme-font:minor-latin'>Import/Phase/from <span
    4234 class=SpellE>RMCProfile</span> .rmc6f file</span></b><span style='mso-fareast-font-family:
    4235 "Times New Roman"'>; a <span class=SpellE>FileDialog</span> box with one entry
    4236 will show the required file, </span><b style='mso-bidi-font-weight:normal'><span
     4213minor-latin;mso-bidi-theme-font:minor-latin'>Import/Phase/from RMCProfile
     4214.rmc6f file</span></b><span style='mso-fareast-font-family:"Times New Roman"'>;
     4215a <span class=SpellE>FileDialog</span> box with one entry will show the
     4216required file, </span><b style='mso-bidi-font-weight:normal'><span
    42374217style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:minor-latin;
    42384218mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:minor-latin;
    … …  
    42664246style='mso-fareast-font-family:"Times New Roman"'> because you don’t want this
    42674247phase to be in any subsequent Rietveld refinement. Looking at the General tab
    4268 for this phase we see it is 6<span class=GramE>,6,4X</span> in all three axes
     4248for this phase we see it is 6x<span class=GramE>,6x,4x</span> in all three axes
    42694249relative to the original and has no symmetry (space group P 1).<o:p></o:p></span></p>
    42704250
    … …  
    42754255 <v:imagedata src="RMCProfile-II_files/image138.png" o:title=""/>
    42764256</v:shape><![endif]--><![if !vml]><img border=0 width=479 height=238
    4277 src="RMCProfile-II_files/image139.gif" v:shapes="Picture_x0020_85"><![endif]></span><span
     4257src="RMCProfile-II_files/image052.gif" v:shapes="Picture_x0020_85"><![endif]></span><span
    42784258style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    42794259
    … …  
    42924272 <v:imagedata src="RMCProfile-II_files/image140.png" o:title=""/>
    42934273</v:shape><![endif]--><![if !vml]><img border=0 width=481 height=452
    4294 src="RMCProfile-II_files/image141.gif" v:shapes="Picture_x0020_86"><![endif]></span><span
     4274src="RMCProfile-II_files/image053.gif" v:shapes="Picture_x0020_86"><![endif]></span><span
    42954275style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    42964276
    42974277<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>NB:
    4298 this import facility can be used to load any rmc6f file, e.g. from a <span
    4299 class=SpellE>RMCProfile</span> run done outside of GSAS-II; all the plotting
    4300 and tools in this and the following steps are available for these big box
    4301 models.<o:p></o:p></span></p>
     4278this import facility can be used to load any rmc6f file, e.g. from a RMCProfile
     4279run done outside of GSAS-II; all the plotting and tools in this and the
     4280following steps are available for these big box models.<o:p></o:p></span></p>
    43024281
    43034282<h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 10. Polyhedral
    … …  
    43204299 <v:imagedata src="RMCProfile-II_files/image142.png" o:title=""/>
    43214300</v:shape><![endif]--><![if !vml]><img border=0 width=477 height=237
    4322 src="RMCProfile-II_files/image143.gif" v:shapes="Picture_x0020_87"><![endif]></span><span
     4301src="RMCProfile-II_files/image054.gif" v:shapes="Picture_x0020_87"><![endif]></span><span
    43234302style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    43244303
    … …  
    43324311 <v:imagedata src="RMCProfile-II_files/image144.png" o:title=""/>
    43334312</v:shape><![endif]--><![if !vml]><img border=0 width=477 height=237
    4334 src="RMCProfile-II_files/image145.gif" v:shapes="Picture_x0020_88"><![endif]></span><span
     4313src="RMCProfile-II_files/image055.gif" v:shapes="Picture_x0020_88"><![endif]></span><span
    43354314style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    43364315
    … …  
    43674346 <v:imagedata src="RMCProfile-II_files/image072.png" o:title=""/>
    43684347</v:shape><![endif]--><![if !vml]><img border=0 width=275 height=234
    4369 src="RMCProfile-II_files/image146.gif" v:shapes="Picture_x0020_38"><![endif]></span><span
     4348src="RMCProfile-II_files/image056.gif" v:shapes="Picture_x0020_38"><![endif]></span><span
    43704349style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    43714350
    … …  
    43984377 <v:imagedata src="RMCProfile-II_files/image147.png" o:title=""/>
    43994378</v:shape><![endif]--><![if !vml]><img border=0 width=481 height=235
    4400 src="RMCProfile-II_files/image149.gif" v:shapes="Picture_x0020_89"><![endif]></span><span
     4379src="RMCProfile-II_files/image057.gif" v:shapes="Picture_x0020_89"><![endif]></span><span
    44014380style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    44024381
    … …  
    44204399 <v:imagedata src="RMCProfile-II_files/image150.png" o:title=""/>
    44214400</v:shape><![endif]--><![if !vml]><img border=0 width=478 height=400
    4422 src="RMCProfile-II_files/image151.gif" v:shapes="Picture_x0020_90"><![endif]></span><span
     4401src="RMCProfile-II_files/image058.gif" v:shapes="Picture_x0020_90"><![endif]></span><span
    44234402style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    44244403
    … …  
    44364415 <v:imagedata src="RMCProfile-II_files/image152.png" o:title=""/>
    44374416</v:shape><![endif]--><![if !vml]><img border=0 width=384 height=103
    4438 src="RMCProfile-II_files/image153.gif" v:shapes="Picture_x0020_91"><![endif]></span><span
     4417src="RMCProfile-II_files/image059.gif" v:shapes="Picture_x0020_91"><![endif]></span><span
    44394418style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    44404419
    … …  
    44524431 <v:imagedata src="RMCProfile-II_files/image154.png" o:title=""/>
    44534432</v:shape><![endif]--><![if !vml]><img border=0 width=624 height=522
    4454 src="RMCProfile-II_files/image155.gif" v:shapes="Picture_x0020_92"><![endif]></span><span
     4433src="RMCProfile-II_files/image060.gif" v:shapes="Picture_x0020_92"><![endif]></span><span
    44554434style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    44564435
    … …  
    44784457<p class=MsoNormal style='tab-stops:344.95pt'><span style='mso-fareast-font-family:
    44794458"Times New Roman";mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_93"
    4480  o:spid="_x0000_i1031" type="#_x0000_t75" style='width:360.75pt;height:302.25pt;
     4459 o:spid="_x0000_i1031" type="#_x0000_t75" style='width:5in;height:303pt;
    44814460 visibility:visible;mso-wrap-style:square'>
    44824461 <v:imagedata src="RMCProfile-II_files/image156.png" o:title=""/>
    4483 </v:shape><![endif]--><![if !vml]><img border=0 width=481 height=403
    4484 src="RMCProfile-II_files/image157.gif" v:shapes="Picture_x0020_93"><![endif]></span><span
     4462</v:shape><![endif]--><![if !vml]><img border=0 width=480 height=404
     4463src="RMCProfile-II_files/image061.gif" v:shapes="Picture_x0020_93"><![endif]></span><span
    44854464style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    44864465
    … …  
    44984477
    44994478<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman";
    4500 mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_94" o:spid="_x0000_i1030"
    4501  type="#_x0000_t75" style='width:358.5pt;height:300pt;visibility:visible;
     4479mso-no-proof:yes'><!--[if gte vml 1]><v:shape id="Picture_x0020_55" o:spid="_x0000_i1030"
     4480 type="#_x0000_t75" style='width:467.25pt;height:292.5pt;visibility:visible;
    45024481 mso-wrap-style:square'>
    4503  <v:imagedata src="RMCProfile-II_files/image158.png" o:title=""/>
    4504 </v:shape><![endif]--><![if !vml]><img border=0 width=478 height=400
    4505 src="RMCProfile-II_files/image159.gif" v:shapes="Picture_x0020_94"><![endif]></span><span
    4506 style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    4507 
    4508 <p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>The
    4509 ‘x’ marks show the directions of the unit vectors about which the TiO<sub>6</sub>
    4510 octahedra are tilted with respect to the reference octahedron. In this case
    4511 they are very tightly distributed; they are clustered about the Z-axis and
    4512 tipped slightly about the Y-axis. <o:p></o:p></span></p>
     4482 <v:imagedata src="RMCProfile-II_files/image062.png" o:title=""/>
     4483</v:shape><![endif]--><![if !vml]><img border=0 width=623 height=390
     4484src="RMCProfile-II_files/image063.gif" v:shapes="Picture_x0020_55"><![endif]></span><span
     4485style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
     4486
     4487<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>What
     4488we see here is a fan of unit vectors along the z-axis all with about the same
     4489color consistent with the tilt angles shown in the right hand panel. About half
     4490are along +Z and the other half along –Z and tipped slightly about the Y-axis. <o:p></o:p></span></p>
    45134491
    45144492<h3><span style='mso-fareast-font-family:"Times New Roman"'>Step 10. View the
    … …  
    45374515 <v:imagedata src="RMCProfile-II_files/image160.png" o:title=""/>
    45384516</v:shape><![endif]--><![if !vml]><img border=0 width=289 height=330
    4539 src="RMCProfile-II_files/image161.gif" v:shapes="Picture_x0020_95"><![endif]></span><span
     4517src="RMCProfile-II_files/image064.gif" v:shapes="Picture_x0020_95"><![endif]></span><span
    45404518style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    45414519
    45424520<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>This
    4543 is the general tool inside GSAS-II for all sorts of structure transformations. Here
    4544 we will use it to push all the big box atoms back into the average structure
    4545 unit cell. Recalling that the big box model is 6x6x4 the original unit cell, we
    4546 simply want to reverse the process. Enter </span><b style='mso-bidi-font-weight:
    4547 normal'><span style='font-family:"Calibri",sans-serif;mso-ascii-theme-font:
    4548 minor-latin;mso-fareast-font-family:"Times New Roman";mso-hansi-theme-font:
    4549 minor-latin;mso-bidi-theme-font:minor-latin'>1/6, 1/6, 1/4</span></b><span
     4521is the general tool inside GSAS-II for all sorts of structure transformations.
     4522Here we will use it to push all the big box atoms back into the average
     4523structure unit cell. Recalling that the big box model is 6x6x4 the original
     4524unit cell, we simply want to reverse the process. Enter </span><b
     4525style='mso-bidi-font-weight:normal'><span style='font-family:"Calibri",sans-serif;
     4526mso-ascii-theme-font:minor-latin;mso-fareast-font-family:"Times New Roman";
     4527mso-hansi-theme-font:minor-latin;mso-bidi-theme-font:minor-latin'>1/6, 1/6, 1/4</span></b><span
    45504528style='mso-fareast-font-family:"Times New Roman"'> into the diagonal elements
    45514529of the M matrix. The GUI will convert them to the decimal equivalent (0.1666
    … …  
    45634541 <v:imagedata src="RMCProfile-II_files/image162.png" o:title=""/>
    45644542</v:shape><![endif]--><![if !vml]><img border=0 width=288 height=329
    4565 src="RMCProfile-II_files/image163.gif" v:shapes="Picture_x0020_96"><![endif]></span><span
     4543src="RMCProfile-II_files/image065.gif" v:shapes="Picture_x0020_96"><![endif]></span><span
    45664544style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    45674545
    … …  
    45854563 <v:imagedata src="RMCProfile-II_files/image164.png" o:title=""/>
    45864564</v:shape><![endif]--><![if !vml]><img border=0 width=624 height=522
    4587 src="RMCProfile-II_files/image165.gif" v:shapes="Picture_x0020_97"><![endif]></span><span
     4565src="RMCProfile-II_files/image066.gif" v:shapes="Picture_x0020_97"><![endif]></span><span
    45884566style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    45894567
    … …  
    46094587 <v:imagedata src="RMCProfile-II_files/image166.png" o:title=""/>
    46104588</v:shape><![endif]--><![if !vml]><img border=0 width=624 height=522
    4611 src="RMCProfile-II_files/image167.gif" v:shapes="Picture_x0020_100"><![endif]></span><span
     4589src="RMCProfile-II_files/image067.gif" v:shapes="Picture_x0020_100"><![endif]></span><span
    46124590style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    46134591
    … …  
    46224600 <v:imagedata src="RMCProfile-II_files/image168.png" o:title=""/>
    46234601</v:shape><![endif]--><![if !vml]><img border=0 width=479 height=401
    4624 src="RMCProfile-II_files/image169.gif" v:shapes="Picture_x0020_101"><![endif]></span><span
     4602src="RMCProfile-II_files/image068.gif" v:shapes="Picture_x0020_101"><![endif]></span><span
    46254603style='mso-fareast-font-family:"Times New Roman"'><o:p></o:p></span></p>
    46264604
    … …  
    46314609<h2><span style='mso-fareast-font-family:"Times New Roman"'>Final note<o:p></o:p></span></h2>
    46324610
    4633 <p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>The
    4634 problem with the value of the <span class=SpellE>difC</span> diffractometer
    4635 constant means that there is an unknown small bias in the scale of G(R) and
    4636 thus all interatomic distances. This is only resolved by careful calibration of
    4637 the diffractometer via known standards using the profile functions known to
    4638 both <span class=SpellE>RMCProfile</span> and GSAS-II and the universal use of
    4639 those parameters for all data reduction steps for both the powder pattern and
    4640 the <span class=GramE>F(</span>Q) and G(R) data sets.<o:p></o:p></span></p>
     4611<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'>The problem
     4612with the value of the <span class=SpellE>difC</span> diffractometer constant
     4613means that there is an unknown small bias in the scale of G(R) and thus all
     4614interatomic distances. This is only resolved by careful calibration of the
     4615diffractometer via known standards using the profile functions known to both
     4616RMCProfile and GSAS-II and the universal use of those parameters for all data
     4617reduction steps for both the powder pattern and the <span class=GramE>F(</span>Q)
     4618and G(R) data sets.<o:p></o:p></span></p>
    46414619
    46424620<p class=MsoNormal><span style='mso-fareast-font-family:"Times New Roman"'><o:p>&nbsp;</o:p></span></p>

  • Tutorials/RMCProfile-II/RMCProfile-II_files/filelist.xml

    r4329 r4358  
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    8  <o:File HRef="image019.gif"/>
     8 <o:File HRef="image002.gif"/>
    99 <o:File HRef="image090.png"/>
    10  <o:File HRef="image021.gif"/>
     10 <o:File HRef="image003.gif"/>
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